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Raman spectroscopy at high temperature has been applied to study in situ the microstructure of the solution in a Cs2O–B2O3–MoO3 growth system. A crystal–solution interface was observed. The BO groups consist of spiral chains based on B3O4Ø2 rings in the solution (Ø is a bridging O atom). The Raman spectrum of the solution indicates that MoO4 tetrahedra existed in the growth system. The nonbridging...
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