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The stretching vibrations of cyanide (CN − ) ions adsorbed on single-crystalline Pt electrodes in aqueous electrolytes were measured in-situ by optical sum-frequency generation (SFG). Adsorption of CN − on well-ordered Pt(111) and Pt(110) surfaces is characterized by a stretching vibration with a strongly potential-dependent frequency, ranging from about 2090 cm −1 near the...
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