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A quarter of a monolayer of carbon monoxide (CO) adsorbs on ethylidyne-covered Pd(111) (ethylidyne saturation coverage, 0.25 monolayers) at 300 K, compared to the saturation coverage of 0.55 monolayers for CO on clean Pd(111). Infrared and temperature-programmed desorption data reveal that CO adsorbs on the hexagonal-close-packed, threefold hollow site on ethylidyne-covered Pd(111). This, in turn,...
The adsorption of methyl isocyanide (CH 3 NC) and acetonitrile (CH 3 CN) has been studied on Pd(111). Methyl isocyanide adsorbs on Pd(111) at 80K at low coverages with the isocyanide functionality oriented close to parallel to the surface; the surface-bound species reorients to a geometry in which the isocyanide group is perpendicular to the surface as the coverage increases. Desorbing...
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