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The development of open‐shell organic molecules that magnetically order at room temperature,which can be practically applied, remains a grand challenge in chemistry, physics, and materials science. Despite the exploration of vast chemical space, design paradigms for organic paramagnetic centers generally result in unpaired electron spins that are unstable or isotropic. Here, a high‐spin conjugated...
Magnetic Ordering
In article number 2206161, Jason D. Azoulay and co‐workers demonstrate that long‐range π‐correlations within a solution‐processed high‐spin conjugated polymer provide robust spin‐centers, intermolecular ferromagnetic exchange interactions, and anisotropic spin ordering. This new approach toward practically applicable metal‐free magnetism opens new opportunities for emerging technologies...
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