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State-resolved two-pulse correlation measurement is useful to study the time scale and mechanism of photo-induced desorption as well as electronic structures of admolecules before desorption. In photodesorption of nitric oxide molecules from Pt(111) at 250 K induced by 80 fs, 620 nm laser pulses, the yields and translational temperatures reached a maximum at zero delay time. In contrast, the rotational...
The electronic and vibrational excitations of single acetylene, pyridine, and benzene molecules on Cu(001) were studied by scanning tunneling microscopy at 9K. Electrons of 0-5eV were used to induce dissociation, desorption, diffusion, rotation, and vibrational excitation of these molecules. The dissociation products were characterized by imaging, single molecule vibrational spectroscopy, and rotational...
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