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A new cobalt(II) complex with a polychlorotriphenylmethyl radical ligand properly functionalized with a carboxylate group (PTMMC−), [Co(PTMMC)2(py)2(H2O)2]·[Co(PTMMC) (py)3(H2O)(Cl)]2·2py·2THF (3), has been synthesized and characterized including single-crystal X-ray diffraction. The structure of 3 consists of two different Co(II) units, [Co(PTMMC)2(py)2(H2O)2] (3A) and [Co(PTMMC) (py)3(H2O)(Cl)]...
The second-order nonlinear optical (SONLO) response of a series of the highly chemically and thermally stable polychlorotriphenylmethyl monoradicals 1–8 has been studied by Hyper-Rayleigh Scattering. These radicals exhibit relatively high nonlinear optical (NLO) responses with β values ranging from 118×10−30 to 755×10−30 esu, which may result from an enhancement of the SONLO activities according to...
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