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We assess the impact of individual experimental observations on a multivariate population balance model for the formation of silicon nanoparticles from the thermal decomposition of silane by means of basic regression influence diagnostics. The nanoparticle model is closely related to one which has been used to simulate soot formation in flames and includes morphological and compositional details which...
This work presents a novel multivariate particle model to simulate the synthesis of silicon nanoparticles across a wide range of process conditions. The gas-phase mechanism of Ho et al. (1994, J. Phys. Chem. 98, 10138–10147) is simultaneously solved with a stochastic population balance incorporated a detailed multidimensional particle model. A systematic parameter estimation procedure is used to adjust...
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