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Doubly charged vanadium–water complexes are produced by laser vaporization in a pulsed supersonic expansion. Size-selected ions are studied with infrared photodissociation spectroscopy in the O–H stretch region using argon complex predissociation. Density functional theory calculations provide structures and vibrational spectra of these ions. The O–H stretches of V 2+ (H 2 O) appear...
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