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Vacancy‐rich layered materials with good electron‐transfer property are of great interest. Herein, a full‐spectrum responsive vacancy‐rich monolayer BiO2−x has been synthesized. The increased density of states at the conduction band (CB) minimum in the monolayer BiO2−x is responsible for the enhanced photon response and photo‐absorption, which were confirmed by UV/Vis‐NIR diffuse reflectance spectra...
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