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An ion-pair complex of [Ni(mnt) 2 ] 2− with p-N-benzylpyridinium α-nitronyl nitroxide radical cations (p-BzPYNN) in acetonitrile shows a moderate and broad absorbance in near-IR region. In the crystal of this complex, two radical cations form a dimer via strong H-bonding interaction; such kinds of dimers are connected into H-bonding chain by [Ni(mnt) 2 ] 2− dianions...
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