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Transition metal tetrylene complexes offer great opportunities for molecular cooperation due to the ambiphilic character of the group 14 element. Here we focus on the coordination of germylene [(ArMes2)2Ge :] (ArMes=C6H3‐2,6‐(C6H2‐2,4,6‐Me3)2) to [RhCl(COD)]2 (COD=1,5‐cyclooctadiene), which yields a neutral germyl complex in which the rhodium center exhibits both η6‐ and η2‐coordination to two mesityl...
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