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Vibrational properties of hydrogen species adsorbed on platinum electrodes in sulfuric acid solution are investigated by visible-infrared Sum-Frequency Generation (SFG). Absolute vibrational spectra are obtained by combining the inherent interfacial selectivity of SFG between centrosymmetric media and the use of a Free Electron Laser (FEL) as a tunable IR source. SFG spectra of hydrogen on polycrystal...
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