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Intracellular dinucleoside polyphosphates (NpnNs) have been known for decades but the functional role remains enigmatic. Diadenosine triphosphate (Ap3A) is one of the most prominent examples, and its intercellular concentration was shown to increase upon cellular stress. By employment of previously reported Ap3A‐based photoaffinity‐labeling probes (PALPs) in chemical proteomics, we investigated the...
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