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Raman spectra of single-phase calcium-silicate hydrate (C-S-H) samples with C/S ratios between 0.88 and 1.45 are consistent with a defect tobermorite model for the structure of these materials, in agreement with previously published nuclear magnetic resonance (NMR) spectroscopic data for the same samples. The Raman spectra of C-S-H samples with C/S ratios <1.0 are very similar to those of 14 ...
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