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Model GaAs(100)/electrolyte interfaces are prepared in vacuum by co‐adsorption of Cl2 and 2‐propanol molecules at LN2 temperature. On adsorption of Cl2 molecules gallium chlorides, elemental arsenic and arsenic chlorides are formed. Co‐adsorption of 2‐propanol causes formation of additional GaCl3 and AsCl, as well as soluble/volatile As‐based complexes, which are released from the surface depleting...
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