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A combined spectroscopic and computational study of gas-phase Au+(CH4)n (n = 3–8) complexes reveals a strongly-bound linear Au+(CH4)2 core structure to which up to four additional ligands bind in a secondary coordination shell. Infrared resonance-enhanced photodissociation spectroscopy in the region of the CH4a1 and t2 fundamental transitions reveals essentially free internal rotation of the core...
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