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Atypically anisotropic and large changes in magnetic susceptibility, along with a change in crystalline shape, were observed in a CoII complex at near room temperature. This was achieved by combining oxalate molecules, acting as rotor, and a CoII ion with unquenched orbital angular momentum. A thermally controlled 90° rotation of the oxalate counter anion triggered a symmetry‐breaking ferroelastic...
Proton transport via dynamic molecules is ubiquitous in chemistry and biology. However, its use as a switching mechanism for properties in functional molecular assemblies is far less common. In this study, we demonstrate how an intra‐carboxyl proton shuttle can be generated in a molecular assembly akin to a rack‐and‐pinion cascade via a thermally induced single‐crystal‐to‐single‐crystal phase transition...
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