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A grand canonical Monte Carlo simulation study of argon adsorption in deformable graphitic slit mesopores has been carried out, to determine the mechanisms of deformation in the different stages of adsorption and desorption. At pressures less than the condensation pressure, especially in the sub-monolayer coverage region, the pore walls are slightly compressed. This is due to the decrease in the potential...
We investigate the effects of the pore cross-section, surface affinity and temperature on argon adsorption in different pore geometries. Three different pore cross sections were considered: cylindrical, hexagonal and triangular. We have placed particular emphasis on the condensation/evaporation (CE) pressures and the behavior of isosteric heat as a function of loading. It was found that CE is not...
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