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The functional core of oxygenic photosynthesis is in charge of catalytic water oxidation by a multi‐redox MnIII/MnIV manifold that evolves through five electronic states (Si , where i=0–4). The synthetic model system of this catalytic cycle and of its S0→S4 intermediates is the expected turning point for artificial photosynthesis. The tetramanganese‐substituted tungstosilicate [MnIII3MnIVO3(CH3COO)...
Der Motor aeroben Lebens auf der Erde ist ein Tetramanganoxokomplex im Zentrum von Photosystem II (PS II) in grünen Pflanzen, Algen und Photosynthesebakterien. In ihrer Zuschrift auf S. 11364 ff. verwenden F. Scandola, U. Kortz, M. Bonchio et al. eine einzigartige Ligandenkombination, um das erste funktionelle Analogon des sauerstoffentwickelnden Komplexes in PS II, das in künstlicher Umgebung funktioniert,...
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