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The dehydrogenation reactions of bimetallic species RhMCH2+ (M=Pt,Rh) with ammonia have been investigated by carrying out density functional calculations. Equilibrium structures and energies have been determined for intermediates and transition states in these reactions. Present results show that both metal–carbene cations have the reactivity similar to that of Pt2CH2+. The variatation of spin multiplicity...
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