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The Monte Carlo method has been used to simulate the kinetic oscillations during partial oxidation of methane under nonisothermal conditions. The oscillatory behavior can be found with the selected parameters by using oxide formation and removal model. From the simulation, the temperature variation during the reaction synchronizes well with the oscillations of product formation rates, and also with...
The Monte Carlo method is employed to study the kinetics of catalytic partial oxidation of methane to syngas on nickel catalyst. Using the Langmuir–Hinshelwood mechanism, self-sustained reaction rate oscillations can be observed under suitable conditions. Further analysis reveals that the rate oscillations are caused by the repetitive oxidation and reduction cycles of nickel surface, which result...
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