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The support effects on the water gas shift reaction activity of [Ru(bpy)(CO)2Cl2] based catalyst were investigated. A series of oxide supports, Al2O3, TiO2, SiO2, Zeolites, ZrO2 and ZrSiO4, was studied. The catalytic activity was significantly improved when the catalyst was supported on weakly acidic alumina.
The effect of a new catalyst activation method on the catalytic activities of several chlorine-containing ruthenium mono(bipyridine) carbonyl complexes in the water–gas shift reaction (WGSR) was studied. The chemical activation of the silica-supported complexes by a sodium carbonate/methanol solution under CO atmosphere produced highly active low-temperature water–gas shift reaction catalysts.
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