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A charge-transfer compound [(CH3)3CNH3]3[PMo12O40] · 2H2O was synthesized and characterized by IR, UV, ESR, diffusion reflectance electronic spectrum, cyclic voltammogram and X-ray crystallography. Oxygen atoms of the polyoxometalate anion, N atoms of organic substrates (CH3)3CNH2 and O atoms of water molecules are involved in hydrogen bonding. The solid reflectance electronic spectra and IR data...
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