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The sequential addition of CN− or CH3− and electrophiles to three perfluoroalkylfullerenes (PFAFs), Cs‐C70(CF3)8, C1‐C70(CF3)10, and Cs‐p‐C60(CF3)2, was carried out to determine the most reactive individual fullerene C atoms (as opposed to the most reactive CC bonds, which has previously been studied). Each PFAF reacted with CH3− or CN− to generate metastable PFAF(CN)− or PFAF(CH3)22− species with...
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