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B3LYP/6‐311+G(3df,2p)//B3LYP/6‐31+G(d,p) density functional theory calculations show that cyclopentene and cyclopentyne derivatives yield very strong π‐type complexes with HCu and FCu molecules. This interaction is so strong in the case of cyclopentyne derivatives that the complexes formed can be considered as a new kind of metallocycles. These complexes resemble those reported before in the literature...
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