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The intracellular second messenger deprotonated adenosine 3′,5′-cyclic monophosphate anion (cAMP-H) − , generated as gaseous species by electrospray ionization (ESI) and stored in a Paul ion-trap mass spectrometer, has been investigated by mass-resolved infrared multiple photon dissociation (IRMPD) spectroscopy in the 900–1800cm −1 fingerprint wavenumber range, exploiting the powerful...
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