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Model catalysts for CO2/epoxide copolymerization based on Co(III) complexes were studied, with focus on the preference of their alternative isomers, cisβ vs. trans. The systems range from model structures without the co‐catalyst, as derived from crystallographic data, to complex models with two (CH2)4N+R3 co‐catalyst chains (R = Me, Bu) grafted onto a Co(III)–salcy core. To explore the conformational...
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