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Ultrathin nickel (Ni)‐based sulfide nanosheets have been reported as excellent electrocatalysts for overall water splitting; however, the uncontrollability over thickness due to the nonlayered structure still hampers its practical application. Herein, a simple topochemical conversion strategy is employed to synthesize cobalt‐doped Ni3S2 (Co‐Ni3S2) ultrathin nanosheets on Ni foam. The Co‐Ni3S2 nanosheets...
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