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Asymmetric bolaamphiphilic sugar-based hydrogelators (1–3) were synthesized and their gelation ability with and without alkylammonium ions was investigated by CD, TEM, FTIR and NMR. These compounds acted as versatile gelators for organic solvents and water. The xerogels 1–3 obtained from water showed well-developed structures of fibrils with diameters of 10–38nm and length of several hundred micrometers...
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