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Silyl ketene acetals and enol ethers are employed as reactive and functional group tolerant nucleophiles in the enantioselective rhodium‐catalyzed alkylative ring opening of a diverse class of oxa/azabicyclic alkenes. This method provides access to enantioenriched dihydronaphthalene and cyclohexene scaffolds, which have the potential to be derivatized toward core motifs of naphthoquinone and sesquiterpene...
Nach einem modularen Ansatz wurden tetrasubstituierte helicale Alkene hergestellt. Dabei ermöglicht eine intermolekulare, Pd‐katalysierte und Norbornen‐vermittelte Dominoreaktion die Bildung dreier C‐C‐Bindungen in einem einzigen Arbeitsschritt über eine Sequenz aus C‐H‐Aktivierung, Carbopalladierung und erneuter C‐H‐Aktivierung.
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