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In an effort to address the need to develop hydrolytically more stable, molecular water reduction catalysts (WRCs) amenable to in-depth investigation, we report here one prototype: a tetra-manganese-containing V-centered polyoxotungstate, Na 10 [Mn 4 (H 2 O) 2 (VW 9 O 34 ) 2 ] (1). The electronic structure of 1 was elucidated using the DFT approach...
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