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Gas‐phase FTIR spectra of the ν6 (B‐type) and the ν4 (C‐type) fundamental bands of S2N2 (D2h) were recorded with a resolution of ≤0.004 cm−1 and the vibrational spectrum of S2N2 (D2h) in solid Ar has been revisited. All IR‐active fundamentals and four combination bands were assigned in excellent agreement with calculated values from anharmonic VPT2 and VCI theory based on (explicitly correlated) coupled‐cluster...
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