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Nitroxide-mediated polymerization enabled the synthesis of cationic, imidazolium-containing triblock copolymers as a membrane for an electromechanical transducer. Nitroxide-mediated polymerization afforded poly(styrene-b-[1-ethyl-3-(4-vinylbenzyl)imidazolium bis(trifluoromethane sulfonyl)imide)]-b-styrene) in a controlled fashion as confirmed using aqueous size exclusion chromatography and 1 ...
Controlled radical polymerization (CRP) allows for the design and synthesis of functional polymers with tailored composition and unique macromolecular architectures. Synthetic methods that are readily available for controlled radical polymerization include nitroxide-mediated polymerization, reversible addition–fragmentation chain transfer polymerization, and atom transfer radical polymerization. N-Vinyl...
The effect of morphology on ion transport in ionic liquid-based solid-state films was investigated. In this study, mixtures of a block copolymer, poly(styrene-b-methyl methacrylate) (SbMMA), and an ionic liquid (IL), 1-ethyl-3-methylimidazolium bis (trifluoromethylsulfonyl)imide (EMIm-TFSI), were prepared as clear solid-state films at various IL compositions (0–50 wt%) by solution casting from a volatile...
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