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Deposition of graphene-like coke during non-oxidative propane dehydrogenation was investigated on a 0.5%Pt/Mg(Al)Ox catalyst. The initial blocking of Pt sites by graphene plays an important role in establishing the excellent steady-state selectivity of Pt-based catalysts toward propylene. Temporal Analysis of Products (TAP) pulse-response experiments was used to demonstrate that during the initial...
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