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Diffusion of water and ethanol in silicalite has been studied in large crystals (70μm×30μm×15μm) synthesized via a fluoride mediated route. The near-perfect hydrophobic silicalite (F − ) crystals have very few internal silanol defects and, as a result, display water and ethanol transport behavior that is uncontaminated by these defects. The transport diffusivity (D t ) of ethanol is...
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