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Nanoscale self‐hosting of spin‐state: Thermally induced spin crossover associated with symmetry breaking yields an unprecedented long‐range ordering in the intermediate (INT) phase (supercell structure of 30 molecules) of a novel molecular material based on an iron complex. A remarkable lozenge pattern is produced, including 12 predominantly high‐spin (HS), 8 predominantly low‐spin (LS), and 10 purely...
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