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Tetraiodoethylene (TIE) forms charge transfer complexes with diazine donors through N...I interactions, in which the structure of the complex is very similar to that of TIE. In TIE, two unique molecules form distinct ''layers'', and in the complexes the donor molecules take the place of TIE molecules in one of the layers. I...I interactions within the remaining layer of TIE maintain the structure...
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