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The magnetic nature of a novel one-dimensional compound NaCr2O4 with zigzag CrO2 chains has been studied by muon spin rotation and relaxation (μ+SR) and neutron diffraction (ND). It is found that NaCr2O4 undergoes an antiferromagnetic transition at TN = 125K, below which the Cr moments in each zigzag chain align ferromagnetically along the c-axis but antiferromagnetically along the a-axis between...
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