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Molecular organization of donor and acceptor chromophores in self‐assembled materials is of paramount interest in the field of photovoltaics or mimicry of natural light‐harvesting systems. With this in mind, a redox‐active porous interpenetrated metal–organic framework (MOF), {[Cd(bpdc)(bpNDI)]⋅4.5 H2O⋅DMF}n (1) has been constructed from a mixed chromophoric system. The μ‐oxo‐bridged secondary building...
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