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The thermal and light‐induced magnetic properties of a family of metal‐diluted spin‐crossover complexes, [FexM1–x(phen)2(NCS)2] (phen = 1,10‐phenantholine and M = NiII, CdII), are reported and compared to previous results obtained for the same series but with ZnII ions used to substitute FeII ions; the ultimate goal was to validate the influence of the size and nature of the inert metal ion on the...
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