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Primary phosphido complexes of aluminum(III) are rare, particularly those that are not supported by interactions with Lewis bases or stabilizing cations. Here we report two new examples of unsupported primary phosphido complexes of Al(III). The ancillary ligand on Al is a pincer ligand, diiminopyridine (denoted as I2P). Solid‐state structures show distorted tetrahedral geometry about Al and single...
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