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The vibrational behaviour of complexes of general formula [(ML5CN)2M′L′4] with either a cis or trans geometry has been studied. The ν(CN) modes have been assigned on the basis of both infrared and Raman intensities. The CN vibrators are but weakly coupled, particularly so in the cis arrangement. The spectroscopic analysis offers insights into the interpretation of the spectra of Prussian Blue species...
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