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This article reports new tris‐cyclometalated IrIII complexes containing mixed‐C^N ligands, (C^N1)2Ir(C^N2), which are a rarely explored class of complexes. Two mixed 2‐phenylpyridine (ppy)/4‐methyl‐2,5‐diphenylpyridine (mdp) complexes (ppy)2Ir(mdp) 3 and (ppy)Ir(mdp)24 have been synthesized and their optoelectronic properties have been systematically characterized. Photoluminescence quantum yield...
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