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Large aqueous ions are interesting because they are useful in materials science (for example to generate thin films) but also because they serve as molecular models for the oxide–aqueous mineral interface where spectroscopy is difficult. Here we show that new clusters of the type M[(μ‐OH)2Co(NH3)4]3(NO3)6 (M=Al, Ga) can be synthesized using Werner's century‐old cluster as a substitutable framework...
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