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AbstractA PtII complex containing N4 bound neutral 1-methylcytosine (1-MeC), trans[Pt(NH3)2(1-MeC-N4)2](ClO4)2 (5), has been prepared and characterized by X-ray analysis. The complex contains the rare iminooxo tautomer form of the cytosine nucleobase. PtII binding is through the exocyclic N4 position of the nucleobases, with Pt and the N3 positions in a syn orientation. As a consequence, the proton...
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