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Introduced approximately two decades ago, macrocyclic deprotonated tetraamido (4N) and, nearly a decade earlier, acyclic diamidodialkoxido or diamidophenolato (2N/2O) ligand systems have been used, among other things, for the synthesis of a wide variety of high-valent complexes of iron, manganese, cobalt, vanadium, nickel, chromium, and copper. Structural, magnetic, and catalytic properties of these...
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