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Time-resolved resonance Raman and infrared spectroscopies have been applied to a variety of problems arising in excited states and molecular assemblies based on polypyridyl complexes of Re(I), Ru(II) and Os(II). Application of transient resonance Raman spectroscopy has been used to assign the acceptor ligand in heteroleptic Ru(II) complexes and to characterize molecular structure in acceptor ligands...
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