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The hydrogenation of a series of linear and cyclic diolefins diluted in decalin, at conditions (≤250 °C, 3.4 MPa H2 and LHSV of 1–2 h−1) chosen to mimic the hydrogenation of a Canadian oil sands naphtha (∼20 wt% olefins and 4–5 wt% diolefins) over a NiMoS/Al2O3 catalyst, is reported. The yield of dimers was minimal on fresh NiMoS/Al2O3 catalyst but increased significantly on spent NiMoS/Al2O3 catalyst...
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