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Self‐folding microscale origami patterns are demonstrated in polymer films with control over mountain/valley assignments and fold angles using trilayers of photo‐crosslinkable copolymers with a temperature‐sensitive hydrogel as the middle layer. The characteristic size scale of the folds W = 30 μm and figure of merit A/W2 ≈ 5000, demonstrated here represent substantial advances in the fabrication...
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