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Topotactic phase transformation enables structural transition without losing the crystalline symmetry of the parental phase and provides an effective platform for elucidating the redox reaction and oxygen diffusion within transition metal oxides. In addition, it enables tuning of the emergent physical properties of complex oxides, through strong interaction between the lattice and electronic degrees...
The real‐time evolution of the electronic phase during the topotactic phase transformation in a SrFeOx thin film is shown. In article number 1606566, Woo Seok Choi and co‐workers report the metal–insulator transition in epitaxial SrFeOx thin films. A pressure–temperature phase diagram of the topotactic transformation is constructed based on real‐time optical spectroscopy and thermodynamic calculation...
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